Lin Wei-Chi, Fang Sin-Kai, Hu Jiun-Wei, Tsai Hsing-Yang, Chen Kew-Yu
Department of Chemical Engineering, Feng Chia University , 40724 Taichung, Taiwan ROC.
Anal Chem. 2014 May 20;86(10):4648-52. doi: 10.1021/ac501024d. Epub 2014 May 9.
A novel salicylideneaniline-based fluorescent sensor, SB1, with a unique excited-state intramolecular charge transfer-excited-state intramolecular proton transfer (ESICT-ESIPT) coupled system was synthesized and demonstrated to fluorescently sense CN(-) with specific selectivity and high sensitivity in aqueous media based on ESICT-ESIPT switching. A large blue shift (96 nm) was also observed in the absorption spectra in response to CN(-). The bleaching of the color could be clearly observed by the naked eye. Moreover, SB1-based test strips were easily fabricated and low-cost, and could be used in practical and efficient CN(-) test kits. Density functional theory (DFT) and time-dependent DFT (TD-DFT) calculations further support the cyanide-induced ESICT-ESIPT switching mechanism. The results provide the proof of concept that the colorimetric and ratiometric fluorescent cyanide-selective chemodosimeter can be created based on an ESICT-ESIPT coupled system.
合成了一种基于水杨醛苯胺的新型荧光传感器SB1,其具有独特的激发态分子内电荷转移-激发态分子内质子转移(ESICT-ESIPT)耦合体系,并基于ESICT-ESIPT开关效应,在水介质中展现出对CN(-)具有特异性选择性和高灵敏度的荧光传感性能。响应CN(-)时,吸收光谱还出现了96 nm的大幅蓝移。肉眼可清晰观察到颜色的褪去。此外,基于SB1的测试条易于制备且成本低廉,可用于实用高效的CN(-)检测试剂盒。密度泛函理论(DFT)和含时密度泛函理论(TD-DFT)计算进一步支持了氰化物诱导的ESICT-ESIPT开关机制。这些结果为基于ESICT-ESIPT耦合体系创建比色和比率荧光氰化物选择性化学计量器提供了概念验证。