Recent advances in dopamine-based materials constructed via one-pot co-assembly strategy.

Dopamine-based materials have attracted widespread interest due to the outstanding physicochemical and biological properties. Since the first report on polydopamine (PDA) films, great efforts have been devoted to develop new fabrication strategies for obtaining novel nanostructures and desirable properties. Among them, one-pot co-assembly strategy offers a unique pathway for integrating multiple properties and functions into dopamine-based platform in a single simultaneous co-deposition step. This review focuses on the state of the art development of one-pot multicomponent self-assembly of dopamine-based materials and summarizes various single-step co-deposition approaches, including PDA-assisted adaptive encapsulation, co-assembly of dopamine with other molecules through non-covalent interactions or covalent interactions. Moreover, emerging applications of dopamine-based materials in the fields ranging from sensing, cancer therapy, catalysis, oil/water separation to antifouling are outlined. In addition, some critical remaining challenges and opportunities are discussed to pave the way towards the rational design and applications of dopamine-based materials.