Koivunen J, Heinonen-Tanski H
Department of Environmental Sciences, University of Kuopio, P.O. Box 1627, FIN-70211 Kuopio, Finland.
Water Res. 2005 Nov;39(18):4445-53. doi: 10.1016/j.watres.2005.08.016. Epub 2005 Oct 10.
The efficiency of peracetic acid (PAA) disinfection against enteric bacteria and viruses in municipal wastewaters was studied in pilot-scale. Disinfection pilot-plant was fed with the primary or secondary effluent of Kuopio municipal wastewater treatment plant or tertiary effluent from the pilot-scale dissolved air flotation (DAF) unit. Disinfectant doses ranged from 2 to 7 mg/l PAA in the secondary and tertiary effluents, and from 5 to 15 mg/l PAA in the primary effluents. Disinfection contact times were 4-27 min. Disinfection of secondary and tertiary effluents with 2-7 mg/l PAA and 27 min contact time achieved around 3 log reductions of total coliforms (TC) and enterococci (EC). PAA disinfection also significantly improved the hygienic quality of the primary effluents: 10-15 mg/l PAA achieved 3-4 log reductions of TC and EC, 5 mg/l PAA resulting in below 2 log reductions. F-RNA coliphages were more resistant against the PAA disinfection and around 1 log reductions of these enteric viruses were typically achieved in the disinfection treatments of the primary, secondary and tertiary effluents. Most of the microbial reductions occurred during the first 4-18 min of contact time, depending on the PAA dose and microorganism. The PAA disinfection efficiency remained relatively constant in the secondary and tertiary effluents, despite of small changes of wastewater quality (COD, SS, turbidity, 253.7 nm transmittance) or temperature. The disinfection efficiency clearly decreased in the primary effluents with substantially higher microbial, organic matter and suspended solids concentrations. The results demonstrated that PAA could be a good alternative disinfection method for elimination of enteric microbes from different wastewaters.
在中试规模下研究了过氧乙酸(PAA)对城市污水中肠道细菌和病毒的消毒效率。消毒中试装置采用库奥皮奥市污水处理厂的一级或二级出水,或中试规模的溶解气浮(DAF)装置的三级出水。二级和三级出水中的消毒剂剂量为2至7mg/L的PAA,一级出水中为5至15mg/L的PAA。消毒接触时间为4至27分钟。用2至7mg/L的PAA对二级和三级出水进行消毒,接触时间为27分钟,可使总大肠菌群(TC)和肠球菌(EC)减少约3个对数级。PAA消毒还显著提高了一级出水的卫生质量:10至15mg/L的PAA可使TC和EC减少3至4个对数级,5mg/L的PAA导致减少量低于2个对数级。F-RNA噬菌体对PAA消毒更具抗性,在一级、二级和三级出水的消毒处理中,这些肠道病毒通常减少约1个对数级。大多数微生物减少发生在接触时间的前4至18分钟,这取决于PAA剂量和微生物。尽管废水质量(化学需氧量、悬浮物、浊度、253.7nm透光率)或温度有小的变化,但PAA在二级和三级出水中的消毒效率保持相对恒定。在微生物、有机物和悬浮固体浓度高得多的一级出水中,消毒效率明显降低。结果表明,PAA可能是从不同废水中消除肠道微生物的一种良好替代消毒方法。