Kim C U, Lew W, Williams M A, Liu H, Zhang L, Swaminathan S, Bischofberger N, Chen M S, Mendel D B, Tai C Y, Laver W G, Stevens R C
Gilead Sciences Inc., Foster City, California 94404, USA.
J Am Chem Soc. 1997 Jan 29;119(4):681-90. doi: 10.1021/ja963036t.
The design, synthesis, and in vitro evaluation of the novel carbocycles as transition-state-based inhibitors of influenza neuraminidase (NA) are described. The double bond position in the carbocyclic analogues plays an important role in NA inhibition as demonstrated by the antiviral activity of 8 (IC50 = 6.3 microM) vs 9 (IC50 > 200 microM). Structure-activity studies of a series of carbocyclic analogues 6a-i identified the 3-pentyloxy moiety as an apparent optimal group at the C3 position with an IC50 value of 1 nM for NA inhibition. The X-ray crystallographic structure of 6h bound to NA revealed the presence of a large hydrophobic pocket in the region corresponding to the glycerol subsite of sialic acid. The high antiviral potency observed for 6h appears to be attributed to a highly favorable hydrophobic interaction in this pocket. The practical synthesis of 6 starting from (-)-quinic acid is also described.
本文描述了新型碳环化合物作为基于过渡态的流感病毒神经氨酸酶(NA)抑制剂的设计、合成及体外评价。碳环类似物中的双键位置在NA抑制中起重要作用,如8(IC50 = 6.3 microM)与9(IC50 > 200 microM)的抗病毒活性所示。一系列碳环类似物6a-i的构效关系研究确定,3-戊氧基部分是C3位置的一个明显最佳基团,对NA抑制的IC50值为1 nM。与NA结合的6h的X射线晶体学结构显示,在对应于唾液酸甘油亚位点的区域存在一个大的疏水口袋。6h观察到的高抗病毒效力似乎归因于该口袋中高度有利的疏水相互作用。还描述了从(-)-奎尼酸出发实际合成6的方法。