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用于宽带光捕获的金纳米盘周期性和随机图案中的表面等离子体共振。

Surface plasmon resonances in periodic and random patterns of gold nano-disks for broadband light harvesting.

作者信息

Nishijima Yoshiaki, Rosa Lorenzo, Juodkazis Saulius

机构信息

Department of Electrical and Computer Engineering, Graduate School of Engineering, Yokohama National University, Hodogaya-ku, Yokohama, Japan.

出版信息

Opt Express. 2012 May 7;20(10):11466-77. doi: 10.1364/OE.20.011466.

Abstract

We analyze the localized surface plasmon resonance spectra of periodic square lattice arrays of gold nano-disks, and we describe numerically and experimentally the effect of disorder on resonance width, spectrum, and EM field enhancement in increasingly randomized patterns. The periodic structure shows a narrower and stronger extinction peak, conversely we observe an increase of up to (1-2)×10(2) times enhancement as the disorder is gradually introduced. This allows for simpler, lower resolution fabrication, cost-effective in light harvesting for solar cell and sensing applications. We show that dipole-dipole interactions contribute to diffract light parallel to the surface as a mean of long-range coupling between the nano-disks.

摘要

我们分析了金纳米盘周期性方形晶格阵列的局域表面等离子体共振光谱,并通过数值和实验描述了无序对共振宽度、光谱以及在逐渐增加的随机图案中电磁场增强的影响。周期性结构呈现出更窄且更强的消光峰,相反,随着无序逐渐引入,我们观察到增强幅度增加了高达(1 - 2)×10²倍。这使得制造过程更简单、分辨率更低,在用于太阳能电池和传感应用的光捕获方面具有成本效益。我们表明,偶极 - 偶极相互作用有助于使光沿与表面平行的方向衍射,这是纳米盘之间长程耦合的一种方式。

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