Duke University, Civil and Environmental Engineering, 121 Hudson Hall, Durham, NC, 27708, USA.
Tsinghua University, School of Architecture, Beijing, 100084, China; Beijing Key Lab of Indoor Air Quality Evaluation and Control, Beijing, 100084, China.
Chemosphere. 2019 Sep;231:256-268. doi: 10.1016/j.chemosphere.2019.05.059. Epub 2019 May 8.
Air pollution in China is an ongoing concern, with subsets of the population (e.g., asthmatic children) especially susceptible to the associated health effects. In addition, people spend the majority of their time indoors, where pollutant composition may differ from the better characterized ambient environment. Although volatile organic compounds (VOCs) present health risks and have high concentrations indoors, their sources have not been thoroughly quantified in typical homes in suburban China. Similarly lacking is an understanding of how well a purifier with high efficiency particulate air and activated carbon filters can remove VOCs in a real-world setting in China. In this study, we a) quantified total VOCs (TVOC) and 900 + individual VOCs in 20 homes in China, b) identified potential sources of VOCs, and c) evaluated impacts of filtration. We used non-negative matrix factorization, a variable reduction technique, to identify sources. TVOC and individual compounds had higher concentrations indoors than outdoors (mean [range] indoors, filtration with pre-filter only: 302 [56-793] μg m; outdoors, entire study: 92 [26-629] μg m), indicating prevalent sources indoors. Many compounds detected have not, to our knowledge, been measured in homes in China. Some compounds (e.g., octanal, heptanal, ⍺-cedrene) were specific to the indoor environment, a few were ubiquitous (e.g., acetaldehyde, formaldehyde), and others were detected infrequently. These compounds may originate from consumer products, solvents, vehicle emissions, a hexane source, wooden products, and cooking. Filtration may improve air quality indoors by lowering concentrations of some VOCs, and, specifically, contributions related to solvents and consumer products.
中国的空气污染问题持续受到关注,某些人群(如哮喘儿童)尤其容易受到相关健康影响。此外,人们大部分时间都在室内度过,而室内污染物的组成可能与特征更为明显的环境有所不同。尽管挥发性有机化合物(VOCs)对健康有风险,且室内浓度较高,但在中国的典型住宅中,其来源尚未得到彻底量化。同样缺乏了解的是,高效微粒空气和活性炭过滤器的空气净化器在现实环境中能在多大程度上去除 VOCs。在这项研究中,我们 a)量化了中国 20 户家庭中的总挥发性有机化合物(TVOC)和 900 多种单个 VOC,b)确定了 VOC 的潜在来源,c)评估了过滤的影响。我们使用非负矩阵分解(一种变量减少技术)来识别来源。TVOC 和个别化合物的室内浓度高于室外(过滤前仅室内[范围]:302[56-793]μg/m;整个研究期间室外:92[26-629]μg/m),表明室内存在普遍的来源。许多检测到的化合物在我们的知识范围内,尚未在中国的家庭中进行测量。一些化合物(例如辛醛、庚醛、α-雪松烯)是室内环境特有的,少数化合物是普遍存在的(例如乙醛、甲醛),其他化合物则很少检测到。这些化合物可能来自消费品、溶剂、车辆排放、己烷源、木制品和烹饪。过滤可能通过降低一些 VOC 的浓度来改善室内空气质量,特别是与溶剂和消费品有关的贡献。