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用于原沉池中微塑料的I型(离散)沉降和上浮的统一建模框架。

A unified modelling framework for type I (discrete) settling and rising of microplastics in primary sedimentation tanks.

作者信息

Sethulekshmi S, Kalbar Pradip, Shriwastav Amritanshu

机构信息

Environmental Science and Engineering Department, Indian Institute of Technology Bombay, Mumbai, 400 076, India.

Centre for Urban Science and Engineering, Indian Institute of Technology Bombay, Mumbai, 400 076, India.

出版信息

J Environ Manage. 2023 May 15;334:117444. doi: 10.1016/j.jenvman.2023.117444. Epub 2023 Feb 9.

Abstract

Sewage treatment plants (STPs) are considered as a significant source of microplastic pollution into the terrestrial and aquatic environment. Existing observations suggest that primary treatment accounts for major microplastics removal in STPs, though with high variability due to the complex nature of the polymer compositions, abundance, and sizes in the incoming sewage. Here, we develop a unified modelling framework to simulate the Type I (or discrete) settling or rising behaviour of microplastics to predict their eventual fate in Primary Sedimentation Tank (PST). The model was developed as per the conventional design protocol for PST involving Stokes equation and modifications as per flow regime for settling of nylon and polystyrene microplastics. It was subsequently validated with independent column experiments for both settling (nylon and polystyrene) and rising (low-density polyethylene and polypropylene) microplastics in different size ranges. The validated model was then applied for multiple realistic scenarios of polymer compositions, relative abundance, and size distributions in the incoming sewage. The model predicts removals ranging from 12% to 94% for a mixture of microplastics in the size fraction 0-500 μm. Model simulations also suggest better microplastics removal with the integration of skimming in PST, and optimization of surface overflow velocity.

摘要

污水处理厂被认为是陆地和水生环境中微塑料污染的一个重要来源。现有观测表明,一级处理是污水处理厂中去除微塑料的主要方式,不过由于进入污水中聚合物成分、丰度和尺寸的复杂性质,去除率存在很大差异。在此,我们开发了一个统一的建模框架,以模拟微塑料的I型(或离散型)沉降或上浮行为,从而预测它们在初沉池中的最终归宿。该模型是根据初沉池的传统设计协议开发的,涉及斯托克斯方程,并根据尼龙和聚苯乙烯微塑料沉降的流态进行了修正。随后,通过独立的柱实验对不同尺寸范围内沉降(尼龙和聚苯乙烯)和上浮(低密度聚乙烯和聚丙烯)微塑料进行了验证。然后将经过验证的模型应用于进水污水中聚合物成分、相对丰度和尺寸分布的多种实际情况。该模型预测,对于尺寸在0 - 500微米范围内的微塑料混合物,去除率在12%至94%之间。模型模拟还表明,通过在初沉池中集成撇渣以及优化表面溢流速度,可以更好地去除微塑料。

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