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一种新型的自由空气柴油与臭氧富集(FADOE)研究平台。

A novel free-air diesel and ozone enrichment (FADOE) research platform.

作者信息

Mofikoya Adedayo O, James Laura, Mullinger Neil J, Ryalls James M W, Girling Robbie D

机构信息

School of Agriculture, Policy and Development, University of Reading, Whiteknights, Earley Gate, Reading RG6 6EU, UK.

School of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham B15 2TT, UK.

出版信息

MethodsX. 2024 Feb 27;12:102635. doi: 10.1016/j.mex.2024.102635. eCollection 2024 Jun.

Abstract

Air pollution is an escalating concern in the modern world, posing substantial threats to ecosystem processes. While the importance of comprehending the impact of pollutants on natural environments is evident, conducting rigorous field-based experiments presents formidable challenges. Elevating pollutant concentrations within open air environments in a controlled manner is complex. Nonetheless, such real-world experiments are invaluable for revealing the genuine influence of air pollutants on ecosystems and their functioning. Field-scale measurements have emerged as a pivotal avenue for advancing our understanding of the interactions between air pollutants and the natural world, providing unique insights into ecosystem dynamics, including critical processes like pollination and natural pest regulation. In atmospheric and ecological research, free-air exposure systems have proven effective in elevating carbon dioxide (CO) and ozone (O) concentrations, facilitating the exploration of their ecological consequences. Yet, nitrogen oxides (NO), a class of pollutants with significant ecological and atmospheric relevance, have largely eluded field-based ecological investigations. This paper introduces the recently developed FADOE (Free-Air Diesel and Ozone Enrichment) platform, which allows the elevation of O and diesel exhaust (including NO) within a field-scale context. Comprehensive information on the system's design, construction, and performance data from the 2023 summer season is presented.•Air pollution and ecosystem functioning•Elevated ozone and nitrogen oxides (NOx)•Free-air exposure systems for field scale measurements.

摘要

空气污染在现代世界中是一个日益严重的问题,对生态系统过程构成了重大威胁。虽然理解污染物对自然环境的影响的重要性是显而易见的,但进行严格的实地实验面临着巨大挑战。以可控方式提高露天环境中的污染物浓度很复杂。尽管如此,这种实际实验对于揭示空气污染物对生态系统及其功能的真正影响非常宝贵。实地尺度的测量已成为增进我们对空气污染物与自然世界之间相互作用理解的关键途径,为生态系统动态提供了独特见解,包括传粉和自然虫害调控等关键过程。在大气和生态研究中,自由空气暴露系统已被证明在提高二氧化碳(CO)和臭氧(O)浓度方面有效,有助于探索其生态后果。然而,氮氧化物(NO),一类具有重要生态和大气相关性的污染物,在很大程度上仍未得到实地生态研究的关注。本文介绍了最近开发的FADOE(自由空气柴油和臭氧富集)平台,该平台可在实地尺度上提高O和柴油尾气(包括NO)的浓度。文中还给出了该系统2023年夏季的设计、构建及性能数据的全面信息。

•空气污染与生态系统功能

•臭氧和氮氧化物(NOx)浓度升高

•用于实地尺度测量的自由空气暴露系统

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8dee/10918276/d7d60f947470/ga1.jpg

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