Department of Biological Sciences, 14 Science drive 4, National University of Singapore, Singapore.
Nucleic Acids Res. 2010 Jul;38(12):4120-32. doi: 10.1093/nar/gkq122. Epub 2010 Mar 1.
Sgm (Sisomicin-gentamicin methyltransferase) from antibiotic-producing bacterium Micromonospora zionensis is an enzyme that confers resistance to aminoglycosides like gentamicin and sisomicin by specifically methylating G1405 in bacterial 16S rRNA. Sgm belongs to the aminoglycoside resistance methyltransferase (Arm) family of enzymes that have been recently found to spread by horizontal gene transfer among disease-causing bacteria. Structural characterization of Arm enzymes is the key to understand their mechanism of action and to develop inhibitors that would block their activity. Here we report the structure of Sgm in complex with cofactors S-adenosylmethionine (AdoMet) and S-adenosylhomocysteine (AdoHcy) at 2.0 and 2.1 A resolution, respectively, and results of mutagenesis and rRNA footprinting, and protein-substrate docking. We propose the mechanism of methylation of G1405 by Sgm and compare it with other m(7)G methyltransferases, revealing a surprising diversity of active sites and binding modes for the same basic reaction of RNA modification. This analysis can serve as a stepping stone towards developing drugs that would specifically block the activity of Arm methyltransferases and thereby re-sensitize pathogenic bacteria to aminoglycoside antibiotics.
来自产抗生素的密旋链霉菌(Micromonospora zionensis)的 Sgm(西索米星-庆大霉素甲基转移酶)是一种酶,通过特异性甲基化细菌 16S rRNA 中的 G1405,赋予对氨基糖苷类抗生素如庆大霉素和西索米星的抗性。Sgm 属于氨基糖苷类抗生素抗性甲基转移酶(Arm)家族的酶,最近发现它们通过水平基因转移在致病细菌之间传播。Arm 酶的结构特征是理解其作用机制和开发阻止其活性的抑制剂的关键。在这里,我们分别以 2.0 和 2.1Å 的分辨率报告了 Sgm 与辅因子 S-腺苷甲硫氨酸(AdoMet)和 S-腺苷同型半胱氨酸(AdoHcy)复合物的结构,以及突变和 rRNA 足迹实验以及蛋白质-底物对接的结果。我们提出了 Sgm 对 G1405 进行甲基化的机制,并将其与其他 m(7)G 甲基转移酶进行了比较,揭示了相同基本 RNA 修饰反应的活性位点和结合模式的惊人多样性。该分析可以作为开发专门阻断 Arm 甲基转移酶活性的药物的垫脚石,从而使致病细菌对氨基糖苷类抗生素重新敏感。