Department of Energy, Environmental, and Chemical Engineering, Washington University in St. Louis, St. Louis, Missouri 63130, United States.
Department of Physics and Atmospheric Science, Dalhousie University, Halifax, Nova Scotia B3H 3J5, Canada.
Environ Sci Technol. 2021 Nov 16;55(22):15287-15300. doi: 10.1021/acs.est.1c05309. Epub 2021 Nov 1.
Annual global satellite-based estimates of fine particulate matter (PM) are widely relied upon for air-quality assessment. Here, we develop and apply a methodology for monthly estimates and uncertainties during the period 1998-2019, which combines satellite retrievals of aerosol optical depth, chemical transport modeling, and ground-based measurements to allow for the characterization of seasonal and episodic exposure, as well as aid air-quality management. Many densely populated regions have their highest PM concentrations in winter, exceeding summertime concentrations by factors of 1.5-3.0 over Eastern Europe, Western Europe, South Asia, and East Asia. In South Asia, in January, regional population-weighted monthly mean PM concentrations exceed 90 μg/m, with local concentrations of approximately 200 μg/m for parts of the Indo-Gangetic Plain. In East Asia, monthly mean PM concentrations have decreased over the period 2010-2019 by 1.6-2.6 μg/m/year, with decreases beginning 2-3 years earlier in summer than in winter. We find evidence that global-monitored locations tend to be in cleaner regions than global mean PM exposure, with large measurement gaps in the Global South. Uncertainty estimates exhibit regional consistency with observed differences between ground-based and satellite-derived PM. The evaluation of uncertainty for agglomerated values indicates that hybrid PM estimates provide precise regional-scale representation, with residual uncertainty inversely proportional to the sample size.
每年基于卫星的细颗粒物(PM)全球估算值被广泛用于空气质量评估。在这里,我们开发并应用了一种方法,用于估算 1998 年至 2019 年期间的月度估算值和不确定性,该方法结合了气溶胶光学深度的卫星反演、化学输送建模和地面测量,以允许描述季节性和偶发性暴露,并有助于空气质量管理。许多人口稠密的地区在冬季的 PM 浓度最高,超过了夏季浓度的 1.5-3.0 倍,涵盖了东欧、西欧、南亚和东亚。在南亚,一月份,区域人口加权月平均 PM 浓度超过 90μg/m,印度河恒河平原部分地区的局部浓度约为 200μg/m。在东亚,2010 年至 2019 年期间,月平均 PM 浓度每年减少了 1.6-2.6μg/m,夏季比冬季早 2-3 年开始减少。我们发现,与全球 PM 暴露相比,全球监测地点往往处于更清洁的区域,而在全球南方,存在大量的测量空白。不确定性估计值与地面和卫星衍生的 PM 之间的观测差异具有区域一致性。对聚集值的不确定性评估表明,混合 PM 估算值提供了精确的区域尺度表示,剩余不确定性与样本大小成反比。