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微塑料在先进饮用水处理厂(ADWTP)中的出现和去除。

Occurrence and removal of microplastics in an advanced drinking water treatment plant (ADWTP).

机构信息

Ministry of Education Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Hohai University, Nanjing 210098, PR China; College of Environment, Hohai University, Nanjing 210098, PR China.

Ministry of Education Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Hohai University, Nanjing 210098, PR China; College of Environment, Hohai University, Nanjing 210098, PR China.

出版信息

Sci Total Environ. 2020 Jan 15;700:134520. doi: 10.1016/j.scitotenv.2019.134520. Epub 2019 Oct 25.

Abstract

Microplastics (MPs) have attracted worldwide attention as the emerging persistent pollutants. Since they have been detected in raw water and the treated water of drinking water treatment plants (DWTPs), there was an urgent need to explore the properties and fates of microplastics in DWTPs. The characteristics of the effluent MPs from each treatment unit in an advanced drinking water treatment plant (ADWTP) were studied, and the relationship between the variations of MPs and the removal performances of treatment processes was also explored. Overall, both the coagulation combined with sedimentation and the granular activated carbon (GAC) filtration performed well in removing microplastics. The former had a removal efficiency of about 40.5-54.5%, mainly for fibres' removal, and the presence of GAC filtration reduced the microplastic abundance by about 56.8-60.9%, mainly for small-sized MPs. It was worthy of attention that a larger amount of polyacrylamide (PAM) was detected in the effluent of the sedimentation compared to raw water, which was caused by the usage of coagulant containing PAM. Specially, the number of 1-5 μm MPs in the effluent of ozonation tank was increased by 2.8-16.0%, resulting in a negative removal efficiency in ozonation. The removals of microplastics were depended primarily on their physical properties (size and shape).

摘要

微塑料(MPs)作为新兴的持久性污染物引起了全球关注。由于它们已经在原水和饮用水处理厂(DWTP)的处理水中被检测到,因此迫切需要探索 DWTP 中微塑料的特性和命运。研究了先进饮用水处理厂(ADWTP)中每个处理单元流出物中的 MPs 特性,并探讨了 MPs 变化与处理工艺去除性能之间的关系。总体而言,混凝沉淀和颗粒活性炭(GAC)过滤都能很好地去除微塑料。前者的去除效率约为 40.5-54.5%,主要用于去除纤维,而 GAC 过滤的存在使微塑料丰度降低了约 56.8-60.9%,主要用于去除小尺寸的 MPs。值得注意的是,与原水相比,沉淀出水中检测到的聚丙烯酰胺(PAM)量较大,这是由于使用了含有 PAM 的混凝剂。特别是,臭氧罐出水中 1-5μm MPs 的数量增加了 2.8-16.0%,导致臭氧处理的去除效率为负。微塑料的去除主要取决于其物理性质(大小和形状)。

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