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全球污水处理厂中微塑料去除的研究综述:特性与机制。

A review of the removal of microplastics in global wastewater treatment plants: Characteristics and mechanisms.

机构信息

Department of Environmental Science and Engineering, Research Centre for Resource and Environment, Beijing University of Chemical Technology, Beijing 100029, People's Republic of China.

Department of Environmental Science and Engineering, Beijing Technology and Business University, Beijing 100048, People's Republic of China.

出版信息

Environ Int. 2021 Jan;146:106277. doi: 10.1016/j.envint.2020.106277. Epub 2020 Nov 20.

Abstract

Wastewater treatment plants (WWTPs) are considered to be the main sources of microplastic contaminants in the aquatic environment, and an in-depth understanding of the behavior of microplastics among the critical treatment technologies in WWTPs is urgently needed. In this paper, the characteristics and removal of microplastics in 38 WWTPs in 11 countries worldwide were reviewed. The abundance of microplastics in the influent, effluent, and sludge was compared. Then, based on existing data, the removal efficiency of microplastics in critical treatment technologies were compared by quantitative analysis. Particularly, detailed mechanisms of critical treatment technologies including primary settling treatment with flocculation, bioreactor system, advanced oxidation and membrane filtration were discussed. Thereafter, the abundance load and ecological hazard of the microplastics discharged from WWTPs into the aquatic and soil environments were summarized. The abundance of microplastics in the influent ranged from 0.28 particles L to 3.14 × 10 particles L, while that in the effluent ranged from 0.01 particles L to 2.97 × 10 particles L. The microplastic abundance in the sludge within the range of 4.40 × 10-2.40 × 10 particles kg. In addition, there are still 5.00 × 10-1.39 × 10 microplastic particles discharged into the aquatic environment each day Moreover, among the critical treatment technologies, the quantitative analysis revealed that filter-based treatment technologies exhibited the best microplastics removal efficiency. Fibers and microplastics with large particle sizes (0.5-5 mm) were easily separated by primary settling. Polyethene and small-particle size microplastics (<0.5 mm) were easily trapped by bacteria in the activated sludge of bioreactor system. The negative impact of microplastics from wastewater treatment plant was worthy of attention. Moreover, unknown transformation products of microplastics and their corresponding toxicity need in-depth research.

摘要

污水处理厂(WWTP)被认为是水环境污染中微塑料污染物的主要来源,因此迫切需要深入了解 WWTP 中关键处理技术中微塑料的行为。本文综述了全球 11 个国家 38 个 WWTP 中微塑料的特征和去除情况。比较了进水、出水和污泥中微塑料的丰度。然后,基于现有数据,通过定量分析比较了关键处理技术中微塑料的去除效率。特别是详细讨论了包括混凝沉淀一级处理、生物反应器系统、高级氧化和膜过滤在内的关键处理技术的详细机制。此后,总结了 WWTP 排放到水和土壤环境中的微塑料的丰度负荷和生态危害。进水微塑料丰度范围为 0.28 个颗粒/L 至 3.14×10 个颗粒/L,而出水微塑料丰度范围为 0.01 个颗粒/L 至 2.97×10 个颗粒/L。污泥中微塑料丰度范围为 4.40×10 -2 至 2.40×10 个颗粒/kg。此外,每天仍有 5.00×10 -1 至 1.39×10 个微塑料颗粒排放到水环境中。此外,在关键处理技术中,定量分析显示基于过滤的处理技术具有最好的微塑料去除效率。纤维和大粒径(0.5-5mm)的微塑料很容易通过一级沉淀分离。聚乙烯和小粒径(<0.5mm)的微塑料很容易被生物反应器系统中活性污泥中的细菌截留。污水处理厂微塑料的负面影响值得关注。此外,需要深入研究微塑料的未知转化产物及其相应的毒性。

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